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Zr-Metal Organic Framework and Derivatives for Adsorptive and Photocatalytic Removal of Acid Dyes

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To investigate effects of modification of MOFs on removal of acid dyes via adsorption and photodegradation, zirconium-based MOF, UiO-66, and its derivatives were synthesized. UiO-66 derivatives were prepared by using amine (NH2)-containing ligand and incorporating carbon nanotubes (CNTs) and reduced graphene oxide (RGO). During the synthesis UiO-66-NH2, UiO-66-CNT and UiO-66-RGO, were obtained, respectively. While UiO-66-NH2 showed the enhanced adsorption capacity for acid dyes owing to the electrostatic attraction, CNTs were found to be the most effective addition to enhance the adsorption of acid dyes. However, the addition of RGO in UiO-66 (to form UiO-66-RGO) exhibited the highest removal efficiency via photodegradation compared to UiO-66 and other derivatives probably attributed to its unique layered morphology. The presence of NH2, CNTs and RGO not only significantly improved the adsorption capacity for acid dyes but also enabled these UiO-66 derivatives to exhibit photocatalytic activity under visible light irradiation.
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Keywords: CNTs; MOFs; UiO-66; acid dyes; graphene; zirconium

Document Type: Research Article

Publication date: 01 February 2018

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    Water Environment Research (WER) publishes peer-reviewed research papers, research notes, state-of-the-art and critical reviews on original, fundamental and applied research in all scientific and technical areas related to water quality, pollution control, and management. An annual Literature Review provides a review of published books and articles on water quality topics from the previous year.

    Published as: Sewage Works Journal, 1928 - 1949; Sewage and Industrial Wastes, 1950 - 1959; Journal Water Pollution Control Federation, 1959 - Oct 1989; Research Journal Water Pollution Control Federation, Nov 1989 - 1991; Water Environment Research, 1992 - present.
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