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Production of H2 and CO from Refuse Derived Fuels Over Ni-Doped CeO2–ZrO2 Catalyst

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Ni-impregnated catalysts, Ni/γ-Al2O3 and Ni/CeO2–ZrO2 (CZO), containing 20 wt.% Ni were used as catalysts for the catalytic reforming, i.e., pyrolysis/gasification, of refuse derived fuels (RDF). In the non-catalytic pyrolysis/gasification of RDF, the amount of syngas was increased with a concomitant increase in H2/CO and CO/CO2 ratios in the syn-gas by applying a higher temperature and equivalence ratio (E/R). In contrast, the catalytic pyrolysis/gasification of RDF over both Ni/γ-Al2O3 and Ni/CZO produced larger amounts of syn-gas than the non-catalytic pyrolysis/gasification of RDF, which was increased further by applying a higher temperature and E/R. By applying a higher temperature and E/R, the H2/CO ratio in the gas product obtained from the catalytic pyrolysis/gasification of RDF was decreased and the CO/CO2 ratio was increased.
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Keywords: NI/CEO2–ZRO2; NI/γ-AL2O3; PYROLYSIS/GASIFICATION; REFUSE DERIVED FUELS; SYN-GAS

Document Type: Research Article

Publication date: September 1, 2018

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  • Science of Advanced Materials (SAM) is an interdisciplinary peer-reviewed journal consolidating research activities in all aspects of advanced materials in the fields of science, engineering and medicine into a single and unique reference source. SAM provides the means for materials scientists, chemists, physicists, biologists, engineers, ceramicists, metallurgists, theoreticians and technocrats to publish original research articles as reviews with author's photo and short biography, full research articles and communications of important new scientific and technological findings, encompassing the fundamental and applied research in all latest aspects of advanced materials.
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