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AMPHI-PIC J-Aggregates: Degree of Disordering and of Thermal Relaxation of Photoproduced Excitons

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Excitonic states in a slightly disordered molecule chain are considered. The chain disordering is modeled through a large number of random realizations related to a given dispersion of disordering. For every random realization, absorption lines are obtained; their averaging over realizations gives the total absorption spectrum. The dispersion of disordering has been evaluated for AMPHI-PIC J-aggregate via matching the calculated absorption spectrum with experimental one. In a similar way luminescence spectrum is considered; it agrees with experiment if calculated under assumption that the population of excitonic levels is almost equilibrium for every random realization.
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Document Type: Research Article

Publication date: 01 September 2005

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  • Journal of Computational and Theoretical Nanoscience is an international peer-reviewed journal with a wide-ranging coverage, consolidates research activities in all aspects of computational and theoretical nanoscience into a single reference source. This journal offers scientists and engineers peer-reviewed research papers in all aspects of computational and theoretical nanoscience and nanotechnology in chemistry, physics, materials science, engineering and biology to publish original full papers and timely state-of-the-art reviews and short communications encompassing the fundamental and applied research.
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