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Structural Aspects, Biological and Nonlinear Optical Response of New N,N–Di(2-tolyl)Formamidinium Tosylate

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N,N –Di(2-tolyl)formamidine (1) was protonated with the aim to explore the structural and solid state properties of the resulting salt. Compound 1 upon protonation with p-toluene sulphonic acid hydrate afforded N,N–Di(2-tolyl)formamidinium tosylate, [1H]+OTs in 90% yield. Compound 1 and [1H]+ OTs were fully characterized by analytical, IR and NMR (1H & 13C) spectroscopic data. The composition of [1H]+OTs was further confirmed by single crystal X-ray diffraction data. The tosylate salt [1H]+OTs crystallized in P21/n space group and exhibited moderate N–H···O and C–H···O hydrogen bonding pattern in the crystal lattice. The thermal stability of [1H]+OTs was evaluated by TGA technique. Both the molecules were found to be moderately active against bacterial strains Staphylococcus aureus, Listeria monocytogenes, Bacillus subtilis, Enterococcus faecalis, Klebsiella pneumoniae, Escherichia coli and Pseudomonas aeruginosa. Further, [1H]+ OTs was evaluated for second harmonic generation response by Kurtz-Perry powder technique.
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Document Type: Research Article

Publication date: June 1, 2013

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  • Advanced Chemistry Letters is an international multidisciplinary peer-reviewed journal covering all fundamental and applied research areas of chemical sciences including organic chemistry, inorganic chemistry, synthetic chemistry, medicinal chemistry, analytical chemistry, organometallic chemistry, nuclear chemistry, electrochemistry, atmospheric chemistry, environmental chemistry, materials chemistry, materials science, supramolecular chemistry, physical chemistry, polymer chemistry, bioinorganic chemistry, physical organic chemistry, surface chemistry, biochemistry, molecular biology, chemical biology, food chemistry, natural product chemistry, neurochemistry, pharmacology, photochemistry, photobiology, toxicology, nanoscience, nanotechnology, agrochemistry, green chemistry, marine chemistry, geochemistry, petrochemistry, radiochemistry, astrochemistry, molecular physics, chemical engineering, quantum chemistry, and theoretical and computational chemistry.
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