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Development of a Household Water Defluoridation Process Using Aluminium Hydroxide Based Adsorbent

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ABSTRACT: 

In this study, the removal of fluoride from water using aluminium hydroxide based adsorbent has been investigated in continuous operation. The effect of fluoride influent concentration, feed flowrate, and adsorbent bed height onto the breakthrough characteristics of the adsorption system were examined. The fixed-bed adsorption system was found to perform better with lower influent fluoride concentration, lower flowrate, and higher bed depth. Thermodynamic evaluation using the bed depth service time model indicated that the fluoride adsorption capacity was 25.8 mg F/g of adsorbent, which is high compared to commercially available activated alumina (1.8 to 1.9 mg/g). Kinetic studies showed that the rate of adsorption in continuous studies was in the range of 6.12 × 10−3 to 39.3 × 10−3 L/mg.h under different operating conditions. The household defluoridation unit (HDU) was tested at an up-flow mode and it was determined that the HDU packed with 0.9 kg of adsorbent with 28.3 cm of bed depth resulted in a specific safe water yield of 823.79 L. Regeneration of the exhaust media using 1% NaOH and 0.1 M HCl showed that the adsorbent could be reused. The estimated running cost of the unit was 2.0 U.S. dollar/m3 of treated water, with the potential to minimize further. Hence, it was concluded that the proposed method is simple and exhibits superior performance for the treatment of fluoride-contaminated water with the potential for household application.
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Keywords: adsorption; fluoride; household defluoridation unit; treated aluminium hydroxide

Document Type: Research Article

Affiliations: Department of Chemistry, Faculty of Science, Addis Ababa University, P.O. Box 1176, Addis Ababa, Ethiopia

Publication date: 01 June 2015

This article was made available online on 09 June 2014 as a Fast Track article with title: "Development of Household Water Defluoridation Process Using Aluminium Hydroxide-Based Adsorbent".

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  • Water Environment Research (WER) is published monthly, including an annual Literature Review. A subscription to WER includes access to the latest content back to 1992, as well as access to fast track articles. An individual subscription is valid for 12 months from month of purchase.

    Water Environment Research (WER) publishes peer-reviewed research papers, research notes, state-of-the-art and critical reviews on original, fundamental and applied research in all scientific and technical areas related to water quality, pollution control, and management. An annual Literature Review provides a review of published books and articles on water quality topics from the previous year.

    Published as: Sewage Works Journal, 1928 - 1949; Sewage and Industrial Wastes, 1950 - 1959; Journal Water Pollution Control Federation, 1959 - Oct 1989; Research Journal Water Pollution Control Federation, Nov 1989 - 1991; Water Environment Research, 1992 - present.
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