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Synthesis, crystal structure and magnetic properties of a novel complex containing a diamagnetic metal ion and thiazole-substituted nitronyl nitroxide radicals

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The synthesis, crystal structure and magnetic properties of a novel diamagnetic metal complex containing thiazole-substituted nitronyl nitroxide radicals, [HgCl2(NIT2-thz)2] (NIT2-thz?= 2-(2'-thiazole)-4,4,5,5-tetramethylimidazoline-1-oxyl-3-oxide), is reported. The mercury(II) ion has distorted tetrahedral coordination involving two chloride atoms and two thiazole nitrogen atoms. Magnetic susceptibility data show that there are intramolecular antiferromagnetic interactions between the radicals in the complex.
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Keywords: Crystal structure; Magnetism; Mercury(II) complex; Nitronyl nitroxide radical

Document Type: Research Article

Affiliations: 1: State Key Laboratory of Coordination Chemistry, Nanjing, 210093, P.R. China 2: Department of Chemistry, Nankai University, Tianjin 300071, P.R. China

Publication date: July 20, 2005

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