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Open Access Time-resolved ARPES at LACUS: Band Structure and Ultrafast Electron Dynamics of Solids

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The manipulation of the electronic properties of solids by light is an exciting goal, which requires knowledge of the electronic structure with energy, momentum and temporal resolution. Time- and angle-resolved photoemission spectroscopy (tr-ARPES) is the most direct probe of the effects of an optical excitation on the band structure of a material. In particular, tr-ARPES in the extreme ultraviolet (VUV) range gives access to the ultrafast dynamics over the entire Brillouin zone. VUV tr-ARPES experiments can now be performed at the ASTRA (ARPES Spectrometer for Time-Resolved Applications) end station of Harmonium, at LACUS. Its capabilities are illustrated by measurements of the ultrafast electronic response of ZrSiTe, a novel topological semimetal characterized by linearly dispersing states located at the Brillouin zone boundary.
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Keywords: ANGLE-RESOLVED PHOTO EMISSION SPECTROSCOPY (ARPES); LACUS; ZRSITE

Document Type: Research Article

Affiliations: 1: Institute of Physics Ecole Polytechnique Fédérale de Lausanne (EPFL) CH-1015 Lausanne 2: Laboratory of Ultrafast Spectroscopy, ISIC and Lausanne Centre for Ultrafast Science (LACUS) Ecole Polytechnique Fédérale de Lausanne (EPFL) CH-1015 Lausanne 3: Institute of Physics Ecole Polytechnique Fédérale de Lausanne (EPFL) CH-1015 Lausanne;, Email: [email protected]

Publication date: 01 May 2017

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  • International Journal for Chemistry and Official Membership Journal of the Swiss Chemical Society (SCS) and its Divisions

    CHIMIA, a scientific journal for chemistry in the broadest sense, is published 10 times a year and covers the interests of a wide and diverse readership. Contributions from all fields of chemistry and related areas are considered for publication in the form of Review Articles and Notes. A characteristic feature of CHIMIA are the thematic issues, each devoted to an area of great current significance.

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