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Methane Oxidation on Perovskite-Type Ca(Mn1−xTix)O3−

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X-ray photoelectron spectroscopy was performed to elucidate the catalytic activity of CH4 oxidation on perovskite-type Ca(Mn1−xTix)O3− synthesized at 1173 K in a flow of oxygen from a gel with citric acid and ethylene glycol. The Mn ion content decreases and the ratio of the Mn3+ ion in the Mn ion increases with increases in x. Ca(Mn1−xTix)O3− has a high catalytic activity of CH4 oxidation at x=0.4. These results indicate that the catalytic activity strongly depends on the Mn3+ ion content of the surface.
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Document Type: Research Article

Affiliations: 1: The Graduate School of Natural Science and Technology (Science), Okayama University, Okayama 700-8530, Japan 2: Kyoto Prefecture Collaboration of Regional Entities for the Advancement of Technological Excellence, Kyoto 619-0237, Japan 3: Faculty of Engineering, Doshisha University, Kyo-tanabe, Kyoto 610-0321, Japan

Publication date: January 1, 2008

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