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Three isomorphous two‐dimensional coordination polymers generated from a benzimidazole bridging ligand and ZnX2 (X = Cl, Br and I)

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A novel bridging asymmetric benzimidazole ligand, 4‐{2‐[3‐(pyridin‐4‐yl)phenyl]‐1H‐benzimidazol‐1‐ylmethyl}benzoic acid, was used to construct three isomorphous two‐dimensional coordination polymers, namely catena‐poly[chlorido(μ3‐4‐{2‐[3‐(pyridin‐4‐yl)phenyl]‐1H‐benzimidazol‐1‐ylmethyl}benzoato)zinc(II)], [Zn(C26H18N3O2)Cl] n , (I), and the bromide, (II), and iodide, (III), analogues. Neighbouring two‐dimensional networks are stacked into three‐dimensional frameworks via interlayer π–π interactions. The luminescent properties of (I)–(III) were investigated and they display an obvious red‐shift in the solid state at room temperature.
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Document Type: Research Article

Affiliations: College of Chemistry, Chemical Engineering and Materials Science, Shandong Normal University, Jinan 250014, People's Republic of China

Publication date: April 15, 2013

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