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Use of Ozone-Based Processes for the Removal of Pharmaceuticals Detected in a Wastewater Treatment Plant

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Abstract:

Ozone (O3)-based processes (O3, O3/H2O2, and O3/UV) were investigated for the removal of pharmaceuticals in real wastewater using a bench-scale experimental setup. An ozone dose of 6 mg/L (contact time  =  10 minutes) was found to reduce the concentration of most pharmaceuticals detected in secondary effluent. Caffeine, N,N-Diethyl-meta-toluamide (DEET), and cyclophosphamide were removed with efficiencies of 84, 89, and 46%, respectively, even with a contact time of 15 minutes (O3 dose  =  6 mg/L). In the case of the ozone process alone, the concentration of bromate ion in the effluent increased with longer contact time. On the other hand, it was found that the O3/H2O2 and O3/UV processes can be used as alternative processes for effective removal of pharmaceuticals, while leaving a low residual concentration of dissolved ozone in the system, thereby preventing bromate formation.

Keywords: advanced oxidation process; bromated; liquid chromatography tandem mass spectrometry (LC/MS/MS); ozone; pharmaceutical

Document Type: Research Article

DOI: http://dx.doi.org/10.2175/106143009X12487095236630

Publication date: April 1, 2010

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  • Water Environment Research® (WER®) publishes peer-reviewed research papers, research notes, state-of-the-art and critical reviews on original, fundamental and applied research in all scientific and technical areas related to water quality, pollution control, and management. An annual Literature Review provides a review of published books and articles on water quality topics from the previous year.

    Published as: Sewage Works Journal, 1928 - 1949; Sewage and Industrial Wastes, 1950 - 1959; Journal Water Pollution Control Federation, 1959 - Oct 1989; Research Journal Water Pollution Control Federation, Nov 1989 - 1991; Water Environment Research, 1992 - present.
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