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Adsorption of Lead(II) from Water by Carbon Nanotubes: Equilibrium, Kinetics, and Thermodynamics

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Abstract:

Adsorption of lead(II) from water on carbon nanotubes (CNTs) was investigated using a series of batch adsorption experiments. The adsorption rate was studied experimentally at various temperatures, contact times, and initial pH and lead(II) concentrations. It was observed that a considerable amount of lead(II) was adsorbed during the first 5 minutes of contact time. The pH of the solution strongly influenced the amount of adsorption, and the best results were obtained when pH value was approximately 6. For the adsorption isotherm, the experimental data were analyzed by three two-parameter isotherms (Langmuir, Freundlich, and Temkin) and four three-parameter isotherms (Redhich-Peterson, Sips, Toth, and Khan). The three kinetic models used to test the experimental data were Lagergren first-order, second-order, and the Elovich equation. The results obtained from the study of the thermodynamic parameters showed that the adsorption of lead(II) onto CNTs was a spontaneous and endothermic process.

Keywords: adsorption isotherm; carbon nanotubes; kinetics; lead; thermodynamic parameter

Document Type: Research Article

DOI: http://dx.doi.org/10.2175/106143008X370511

Affiliations: Chemical Engineering Department, Shahid Bahonar University, Kerman, Iran.

Publication date: June 1, 2009

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  • Water Environment Research® (WER®) publishes peer-reviewed research papers, research notes, state-of-the-art and critical reviews on original, fundamental and applied research in all scientific and technical areas related to water quality, pollution control, and management. An annual Literature Review provides a review of published books and articles on water quality topics from the previous year.

    Published as: Sewage Works Journal, 1928 - 1949; Sewage and Industrial Wastes, 1950 - 1959; Journal Water Pollution Control Federation, 1959 - Oct 1989; Research Journal Water Pollution Control Federation, Nov 1989 - 1991; Water Environment Research, 1992 - present.
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