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Lanthanide Luminescence Spectroscopy as a Monitor of Crystal Structure

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Abstract:

We wish to address the criticisms of Tanner and Rudowicz regarding the feasibility of using lanthanide luminescence spectroscopy as a monitor of crystal structure, as was suggested in the recent paper by Chen et al. Such optical methods (including absorption and phonon Raman spectroscopy) have been and continue to be employed successfully by the present authors to investigate and characterize f-element solids. The ability to use such methods to recognize structures is a matter of record; to argue their nonfeasibility rejects this past evidence and success.

Keywords: Eu3+ ion luminescence; Lanthanide sesquioxides; Optical probe of structure

Document Type: Short Communication

DOI: http://dx.doi.org/10.1366/0003702934065902

Affiliations: 1: Department of Chemistry, University of Tennessee, Knoxville, Tennessee 37996-1600 2: Transuranium Research Laboratory (Chemistry Division), Oak Ridge National Laboratory, P.O. Box 2008, Oak Ridge, Tennessee 37831-6375 3: Department of Chemistry, University of Tennessee, Knoxville, Tennessee 37996-1600; Transuranium Research Laboratory (Chemistry Division), Oak Ridge National Laboratory, P.O. Box 2008, Oak Ridge, Tennessee 37831-6375

Publication date: November 1, 1993

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