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Recent Developments in Two-Dimensional Infrared (2D IR) Correlation Spectroscopy

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Recent developments in two-dimensional infrared (2D IR) correlation spectroscopy are reviewed. Since the initial introduction of the basic concept seven years ago, the field of 2D IR spectroscopy has evolved considerably. The method for generating 2D IR spectra from perturbation-induced time-dependent fluctuations of IR intensities and the properties of such 2D spectra are summarized first. Applications of 2D IR spectroscopy are then surveyed, and improvements in the instrumentation are reviewed. Different types of external perturbation schemes capable of inducing dynamic fluctuations of IR spectra are listed. Finally, a new 2D correlation method for dynamic spectral data with arbitrary time-dependence is discussed.

Keywords: 2D IR spectroscopy; Correlation spectra; Fourier transform; Infrared; Review; Spectroscopic technique; Time-resolved spectroscopy; Two-dimensional spectroscopy

Document Type: Invited Paper

DOI: http://dx.doi.org/10.1366/0003702934067513

Affiliations: The Procter and Gamble Company, Miami Valley Laboratories, P.O. Box 398707, Cincinnati, Ohio 45239-8707

Publication date: September 1, 1993

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