On the Phase Match in Multiplex CARS of Condensed Media

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The phase-matching conditions in condensed-media multiplex CARS are analyzed for the case where a spectral region is recorded according to variation of the pump frequency. The possibility of eliminating the influence of the phase mismatch on the recorded CARS spectra and of experimentally evaluating the third-order electronic susceptibility tensor is discussed.

Keywords: CARS; Nonlinear susceptibility; Phase match

Document Type: Research Article

DOI: http://dx.doi.org/10.1366/0003702934334985

Affiliations: Institute of Solid State Physics, Blvd. "Tzarigradsko Chaussee" 72, Sofia 1784, Bulgaria

Publication date: April 1, 1993

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