Fourier Transform Infrared Spectrometry Using a Very-Long-Pathlength Cell: Dioxygen Difluoride Stability and Reactions with Plutonium Compounds

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Abstract:

A unique spectroscopic device combining a Fourier transform infrared spectrometry instrument and a very-long-pathlength cell (a few hundred meters) is described. It shows much promise for spectroscopic studies of unstable or transient species at extremely low concentrations in a temperature-controlled environment. Results are presented of dioxygen difluoride (O2F2) fluorination reactions with Pu compounds and of O2F2 thermal stability measurements in the cell.

Keywords: Infrared; Interferometry, infrared region; Spectroscopic techniques

Document Type: Research Article

DOI: http://dx.doi.org/10.1366/0003702854250284

Affiliations: Los Alamos National Laboratory, Los Alamos, New Mexico 87545

Publication date: July 1, 1985

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