Closed-Form Calculation of Coherent Anti-Stokes Raman and Stimulated Raman Scattering Spectral Profiles

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The third-order susceptibility is expressed as a summation of interfering resonant terms, each involving the phenomenological linewidth of the transition. Correlations of the finite line-width of the laser sources with |X (3)|2 (coherent anti-Stokes Raman spectroscopy) and –X" (stimulated Raman scattering) are performed and closed-form expressions for the theoretical profiles are obtained.

Keywords: Raman spectroscopy

Document Type: Research Article


Affiliations: Arnold Engineering and Development Center, Tullahoma, Tennessee 37389

Publication date: May 1, 1981

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