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Mass Spectrometric Observation of Polymers of Carbon Dioxide in a Molecular Beam System

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The operation of a mass spectrometer equipped with a molecular beam gas sampling system is described. Polymeric ions, (CO2)n + where n varies from two to twelve, are observed when sampling CO2 at 1 to 6.5 atm; similar polymers are found in SO2 and N2O. A possible explanation is advanced in terms of isentropic expansion in the sampling process and subsequent condensation.

Document Type: Research Article

DOI: http://dx.doi.org/10.1366/000370265789620078

Affiliations: Chemistry Division, A.E.R.E., Harwell, Berkshire, England

Publication date: January 1, 1965

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