Magnetic properties and the phase diagram of La [iopmath latex="$_{1-x}$"] 1-x [/iopmath] Sr [iopmath latex="$_{x}$"] x [/iopmath] MnO3 for [iopmath latex="$x \leq0.2$"] x0.2 [/iopmath]

Authors: Paraskevopoulos M.1; Mayr F.1; Hemberger J.1; Loidl A.1; Heichele R.2; Maurer D.2; Mller V.2; Mukhin A.A.3; Balbashov A.M.4

Source: Journal of Physics: Condensed Matter, Volume 12, Number 17, 2000 , pp. 3993-4011(19)

Publisher: Institute of Physics Publishing

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Abstract:

We report on susceptibility, magnetization, magnetoresistance, and ultrasonic studies of La [iopmath latex="$_{1-x}{\rm Sr}_{x}{\rm MnO}_{3}$"] 1-xSrxMnO3 [/iopmath] for [iopmath latex="$x\leq 0.2$"] x0.2 [/iopmath] . The magnetic susceptibilities in the different high-temperature paramagnetic phases are studied in detail. We provide experimental evidence for the occurrence of short-range ferromagnetic order within the paramagnetic phase. Furthermore, we can exclude the possibility of electronic phase separation for [iopmath latex="$x\lt 0.1$"] x<0.1 [/iopmath] . Variable-range-hopping conductivity dominates in the paramagnetic and magnetically ordered phases. From the anomalies at the structural and magnetic phase transitions, we arrive at a phase diagram which shows a ferromagnetic and insulating ground state for [iopmath latex="$0.1\leq x\leq 0.15$"] 0.1x0.15 [/iopmath] , followed by a canted antiferromagnetic phase at higher temperatures. The ferromagnetic transition is strongly coupled to a structural transition from a Jahn-Teller-distorted phase to a pseudocubic orthorhombic phase and is accompanied by the appearance of large positive magnetoresistance effects. We interpret the rich phase diagram close to [iopmath latex="$x=1/8$"] x = 1/8 [/iopmath] in terms of orbital ordering, due to an interplay of superexchange interactions and Jahn-Teller distortions.

Language: English

Document Type: Miscellaneous

Affiliations: 1: Experimentalphysik V, Elektronische, Korrelationen und Magnetismus, Institut f?r Physik, Universit?t Augsburg, D-86159 Augsburg, Germany 2: Experimentalphysik III, Institut f?r Physik, Universit?t Augsburg, D-86159 Augsburg, Germany 3: Moscow Power Engineering Institute, 105835 Moscow, Russia 4: General Physics Institute of the Russian Academy of Sciences, 117942 Moscow, Russia

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