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Effects of Frequency, Percolation, and Axisymmetric Microstructure on the Electrical Response of Hot-Pressed Alumina–Silicon Carbide Whisker Composites

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Abstract:

The electrical and dielectric properties of hot-pressed composites containing alumina and silicon carbide (SiC) whiskers were characterized over a wide frequency range (0.1 Hz–1.8 GHz). The results were correlated to the average distances between SiC inclusions which were measured by stereology as a function of orientation and composition. Percolation of the whiskers caused a drastic increase in the dc conductivity and the prominence of a dc-conductivity tail associated with a high-frequency Maxwell–Wagner interfacial polarization. In percolated samples, the tail obscured the dielectric loss peak and there was evidence for the fluctuation-induced tunneling mechanism of conduction. In nonpercolated samples, the loss peak was observed and the complex permittivity data were fit with a modified Maxwell–Wagner equation to account for a distribution of relaxation times. The frequency–dispersion magnitudes, fitting exponents, and central relaxation times were orientation-dependent. Also, a damped resonance was observed between 1.4 and 1.7 GHz. The influence of the results on the microwave-heating application is discussed.

Document Type: Research Article

DOI: http://dx.doi.org/10.1111/j.1551-2916.2010.04156.x

Affiliations: School of Materials Science and Engineering, Georgia Institute of Technology, Atlanta, Georgia 30332-0245

Publication date: April 1, 2011

bsc/jace/2011/00000094/00000004/art00030
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