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Ligandless Copper‐Catalyzed Coupling of Heteroaryl Bromides with Gaseous Ammonia

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Abstract

A range of different N‐ and S‐containing heterocyclic bromides can be efficiently coupled with gaseous ammonia in the presence of copper(II) acetylacetonate [Cu(acac)2] as catalyst and in the absence of additional ligands. Unstable aminothiophenes and aminobenzothiophenes can be further reacted in situ to afford functionalized derivatives.
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Document Type: Communications

Affiliations: Process Research & Synthesis, F. Hoffmann-La Roche Ltd, 4070 Basel, Switzerland, phone: (+41)-61-687-7396, Fax: (+41)-61-688-1670

Publication date: 2013-03-11

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