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Arylboronic Acid-Lead Tetraacetate-Copper Diacetate: A One-Pot System for Copper-Catalyzed N-Arylation Under Neutral Conditions

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Abstract:

The one-pot reaction of arylboronic acids with lead tetraacetate in chloroform followed by treatment with 3,4-dimethylaniline in the presence of catalytic copper diacetate gave the corresponding diarylamines under neutral conditions in good to high yields. The reaction proceeded with electron-rich as well as with electron-depleted arylboronic derivatives.

Keywords: arylboronic acid; aryllead triacetate; copper diacetate catalysis; diarylamines; ullmann-modified N-arylation

Document Type: Review Article

DOI: http://dx.doi.org/10.2174/1570178054405995

Affiliations: Laboratoire de Valorisation de la Chimie Fine, UMR CNRS 6178; Universite Paul Cezanne - Case 552; Faculte des Sciences St Jerome, 13397 Marseille Cedex 20, France;

Publication date: August 1, 2005

More about this publication?
  • Letters in Organic Chemistry publishes original letters on all areas of organic chemistry including synthesis, bioorganic, medicinal, natural products, organometallic, supramolecular, molecular recognition and physical organic chemistry. The emphasis is placed on publishing quality papers very rapidly. Letters are processed rapidly and take full advantage of the Internet technology both for the submission and the review of the manuscripts.
    The journal is essential reading for all organic chemists both in academia and industry.
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