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Finite-Difference Time-Domain Numerical Simulation Study on the Optical Properties of Silver Nanocomposites

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Abstract:

The effects of the nanoparticle geometry and the host matrix on the optical properties of silver (Ag) nanocomposites were investigated. The spatial intensity distribution and absorption spectra were obtained by solving Maxwell equations using the finite-difference time-domain method. Local enhancement of the optical field was produced near the surface of the Ag nanoparticle. As the nanoparticle size increased, the plasmon-induced absorption increased and the surface plasmon resonance (SPR) wavelength of the Ag nanocomposite was redshifted. As the nanoparticle geometry was transformed from a sphere to an ellipsoid, two plasmon peaks appeared and their spectral spacing became larger with increasing the aspect ratio. The effects of the nanoparticle size and the anisotropic geometry on the optical properties of the Ag nanocomposites can be described by the Maxwell-Garnett theory and the Drude model. From the absorption spectra of the Ag nanocomposites with five different host matrices (SiO2, Al2 O3, ZnO, ZrO2, and TiO2[U+0002], it was found that the SPR wavelength of the Ag nanocomposite was redshifted with increasing the refractive index of the host matrix.

Document Type: Research Article

DOI: http://dx.doi.org/10.1166/jnn.2012.6330

Publication date: July 1, 2012

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  • Journal for Nanoscience and Nanotechnology (JNN) is an international and multidisciplinary peer-reviewed journal with a wide-ranging coverage, consolidating research activities in all areas of nanoscience and nanotechnology into a single and unique reference source. JNN is the first cross-disciplinary journal to publish original full research articles, rapid communications of important new scientific and technological findings, timely state-of-the-art reviews with author's photo and short biography, and current research news encompassing the fundamental and applied research in all disciplines of science, engineering and medicine.
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