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Enhancing the Photoelectric Conversion of Dye-Sensitized Solar Cell via Nitrogen-Doped Nanocrystalline Titania Electrode

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A high efficient dye-sensitized solar cell (DSC) was fabricated using nitrogen-doped nanocrystalline titania(TiO2) photoanode. X-ray photoelectron spectroscopy (XPS), diffuse reflectance spectroscopy (DRS), X-ray powder diffraction (XRD), zeta potentials, nitrogen adsorption–desorption and elemental analysis experiments were employed to characterize the nitrogen-doped nanocrystalline TiO2 photoanode. An obvious enhancement of the optical absorption in the range of 380–550 nm was observed for nitrogen-doped TiO2, which was attributed to both the substitutional N and the chemisorbed N2 molecules. A conversion efficiency of 9.04% was obtained on the DSC based on nitrogen-doped TiO2 photoanode annealed in a flow of NH3 at 550 °C, with an increase of 15.6% improvement in comparison with pure TiO2 (7.82%). The mechanism for the enhanced photovoltaic performance was discussed.
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Keywords: DYE-SENSITIZED SOLAR CELL; NITROGEN-DOPED; PHOTOVOLTAIC PERFORMANCE; TITANIA

Document Type: Research Article

Publication date: 2010-11-01

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  • Journal for Nanoscience and Nanotechnology (JNN) is an international and multidisciplinary peer-reviewed journal with a wide-ranging coverage, consolidating research activities in all areas of nanoscience and nanotechnology into a single and unique reference source. JNN is the first cross-disciplinary journal to publish original full research articles, rapid communications of important new scientific and technological findings, timely state-of-the-art reviews with author's photo and short biography, and current research news encompassing the fundamental and applied research in all disciplines of science, engineering and medicine.
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