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Large Third-Order Optical Nonlinearity in Directly Synthesized Single-Walled Carbon Nanotube Films

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Abstract:

Large third-order optical nonlinearity is observed in single-walled carbon nanotube (SWNT) films that are directly synthesized by CVD method rather than post-deposited from solution. Through z-scan method, the third-order nonlinear susceptibility ((3)) is measured, and the |Im(3)| is 1.8 × 10−7 esu at 1064 nm, which is among the highest reported values for optical nonlinear materials. Combined with their transparent morphology and ultrafast carrier relaxation time, our results indicate the promising prospect of directly synthesized SWNT films as saturable absorbers using in mode-lock lasers or ultrafast switching materials in optical telecommunications.

Keywords: NONLINEAR OPTICS; SATURABLE ABSORBER; SINGLE-WALLED CARBON NANOTUBE

Document Type: Research Article

DOI: https://doi.org/10.1166/jnn.2010.2913

Publication date: 2010-11-01

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  • Journal for Nanoscience and Nanotechnology (JNN) is an international and multidisciplinary peer-reviewed journal with a wide-ranging coverage, consolidating research activities in all areas of nanoscience and nanotechnology into a single and unique reference source. JNN is the first cross-disciplinary journal to publish original full research articles, rapid communications of important new scientific and technological findings, timely state-of-the-art reviews with author's photo and short biography, and current research news encompassing the fundamental and applied research in all disciplines of science, engineering and medicine.
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