Electric Field Directed Layer-by-Layer Assembly of Highly Fluorescent CdTe Nanoparticles
Abstract:An electric field directed layer-by-layer assembly technique has been developed by combining electrophoretic deposition and the layer-by-layer self-assembly method. This technique is employed to realize spatially selective deposition of CdTe nanoparticles on electrodes of indium–tin oxide (ITO). The fluorescence measurements prove that the selectivity of the film deposition increases against applied voltage and reaches 99% when the voltage is 1.4 V. Upon further increase of the voltage, the selectivity slightly decreases. This decrease occurs because high voltage leads to a degradation of CdTe particles and thus reduces fluorescence intensity of the resultant CdTe film. However, fluorescence investigation indicates that a spacer layer of polyelectrolyte complex between the ITO electrode and the CdTe film is useful to protect the CdTe from being destroyed under high voltages.
Document Type: Communications
Affiliations: Department of Physics and Center of Nanoscience, University of Munich, Amalienstrasse 54, D-80799 Munich, Germany
Publication date: June 1, 2001
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