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Photodegradation of SiO2-Coated CdS Nanoparticles within Silica Gels

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A comparative study of the photodegradation of CdS nanoparticles coated with silica shells dispersed in water and embedded in two silica gels with different pore size is presented. Although encapsulation of the quantum dots in a silica shell previously was proven to provide a basically permanent protection against light-induced surface oxidation (photodegradation), this protection is not always maintained when the coated particles are incorporated within different silica gels. Degradation of the CdS occurs when the coated particles are incorporated within silica gels with an open structure, which suggests that the shells somehow crack due to tension in the gel structure. This behavior is analyzed by absorption and luminescence spectroscopies, electron microscopy, and nitrogen sorption.
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Keywords: CDS; GELS; NANOPARTICLES; PHOTODEGRADATION; QUANTUM DOTS; SILICA

Document Type: Research Article

Affiliations: 1: Departemento de Química Física, Universidade de Vigo, 36200 Vigo, Spain 2: Max Planck Institute of Colloids and Interfaces, D-14424 Potsdam, Germany

Publication date: 01 March 2001

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  • Journal for Nanoscience and Nanotechnology (JNN) is an international and multidisciplinary peer-reviewed journal with a wide-ranging coverage, consolidating research activities in all areas of nanoscience and nanotechnology into a single and unique reference source. JNN is the first cross-disciplinary journal to publish original full research articles, rapid communications of important new scientific and technological findings, timely state-of-the-art reviews with author's photo and short biography, and current research news encompassing the fundamental and applied research in all disciplines of science, engineering and medicine.
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