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Diamondoids-DNA Nanoarchitecture: From Nanomodules Design to Self-Assembly

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Abstract:

Diamondoids are one of the promising molecular building blocks (MBBs) proposed for the fabrication of a diverse range of nanostructures in molecular nanotechnology and manufacturing. The challenge is to find a route for self-assembly of these cage hydrocarbons and their application in the bottom-up synthesis. In this context, we propose a DNA-based self-assembly technique called "DNA Bridge-based Self-assembly" (DBS) to self-assemble the diamondoid molecules based upon a bottom-up strategy. The idea supporting the hypothesis is based on the well-established proofs of DNA-based self-assembly. Furthermore, the previous findings in the field of DNA nanotechnology would be inspiring to develop DBS for the construction of Diamondoid-DNA-made nanoarchitecture. The results of our computations and simulations with different molecular mechanical force fields (MM+, AMBER, BIO+, and OPLS) and different optimization algorithms (Polak-Ribiere, Fletcher-Reeves, and block-diagonal Newton-Raphson) furthermore confirm the feasibility of the formation of such hybrid nanoarchitecture.

Keywords: BOTTOM-UP SYNTHESIS; DIAMONDOIDS; DNA BRIDGE-BASED SELF-ASSEMBLY (DBS); DNA NANOTECHNOLOGY; SELF-ASSEMBLY

Document Type: Research Article

DOI: http://dx.doi.org/10.1166/jctn.2007.008

Publication date: February 1, 2007

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  • Journal of Computational and Theoretical Nanoscience is an international peer-reviewed journal with a wide-ranging coverage, consolidates research activities in all aspects of computational and theoretical nanoscience into a single reference source. This journal offers scientists and engineers peer-reviewed research papers in all aspects of computational and theoretical nanoscience and nanotechnology in chemistry, physics, materials science, engineering and biology to publish original full papers and timely state-of-the-art reviews and short communications encompassing the fundamental and applied research.
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